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Cheng, Shan-Wen; Xu, Ding; Su, Haowen; Baxter, James M; Holtzman, Luke N; Watanabe, Kenji; Taniguchi, Takashi; Hone, James C; Barmak, Katayun; Delor, Milan (, Nano Letters)
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Xu, Ding; Mandal, Arkajit; Baxter, James M.; Cheng, Shan-Wen; Lee, Inki; Su, Haowen; Liu, Song; Reichman, David R.; Delor, Milan (, Nature Communications)Abstract Semiconductor excitations can hybridize with cavity photons to form exciton-polaritons (EPs) with remarkable properties, including light-like energy flow combined with matter-like interactions. To fully harness these properties, EPs must retain ballistic, coherent transport despite matter-mediated interactions with lattice phonons. Here we develop a nonlinear momentum-resolved optical approach that directly images EPs in real space on femtosecond scales in a range of polaritonic architectures. We focus our analysis on EP propagation in layered halide perovskite microcavities. We reveal that EP–phonon interactions lead to a large renormalization of EP velocities at high excitonic fractions at room temperature. Despite these strong EP–phonon interactions, ballistic transport is maintained for up to half-exciton EPs, in agreement with quantum simulations of dynamic disorder shielding through light-matter hybridization. Above 50% excitonic character, rapid decoherence leads to diffusive transport. Our work provides a general framework to precisely balance EP coherence, velocity, and nonlinear interactions.more » « less
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Xu, Ding; Mandal, Arkajit; Baxter, James M.; Cheng, Shan-Wen; Lee, Inki; Su, Haowen; Liu, Song; Reichman, David R.; Delor, Milan (, ArXivorg)
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